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dc.creatorFaroldi, Betina María Cecilia-
dc.creatorIrusta, Silvia-
dc.creatorCornaglia, Laura Maria-
dc.date2018-01-30T15:48:36Z-
dc.date2018-01-30T15:48:36Z-
dc.date2015-09-
dc.date2018-01-18T14:39:29Z-
dc.date.accessioned2019-04-29T15:41:48Z-
dc.date.available2019-04-29T15:41:48Z-
dc.date.issued2015-09-
dc.identifierFaroldi, Betina María Cecilia; Irusta, Silvia; Cornaglia, Laura Maria; Influence of La incorporation on the catalytic activity of Ru/ETS-10 catalysts for hydrogen production; Elsevier; Applied Catalysis A: General; 504; 9-2015; 391-398-
dc.identifier0926-860X-
dc.identifierhttp://hdl.handle.net/11336/34989-
dc.identifierCONICET Digital-
dc.identifierCONICET-
dc.identifier.urihttp://rodna.bn.gov.ar:8080/jspui/handle/bnmm/299785-
dc.descriptionThe incorporation of lanthanum on ETS-10 titanosilicate and its influence on the catalytic activity of Ru catalysts for the dry reforming of methane reaction were studied. The catalysts were prepared through ion exchange of ETS-10 using different lanthanum solution concentrations (0.1, 0.2 and 0.4 % wt of La2O3). The Ru loading was 0.6 wt.% for all catalysts. The methane reaction rates for Ru/LaETS-10 catalysts showed an increase in comparison with Ru/ETS-10. This could be related to the lanthanum participation in the reaction mechanism. Moreover, all the formulations were stable after 70 h on stream. In order to study the effect of lanthanum exchange in the structure of ETS-10 supports, the solids were characterized by BET, XRD, TEM, FTIR XPS, and Laser Raman spectroscopy. The relative crystallinities were lower than 80%, indicating that the La exchange could have an important effect on the crystalline structure of ETS-10, in agreement with Raman and FTIR results. The surface Ru/Ti ratio determined by XPS was higher in the case of Ru/LaETS-10 synthesized with the highest La concentration in the exchange solution. The Na/Ti ratio, measured by XPS and EDX, was lower for the Ru/LaETS-10 catalysts compared with ETS-10 suggesting that La was exchanged in the structure.-
dc.descriptionFil: Faroldi, Betina María Cecilia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica ; Argentina-
dc.descriptionFil: Irusta, Silvia. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España-
dc.descriptionFil: Cornaglia, Laura Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica ; Argentina-
dc.formatapplication/pdf-
dc.formatapplication/pdf-
dc.languageeng-
dc.publisherElsevier-
dc.relationinfo:eu-repo/semantics/altIdentifier/doi/https://doi.org/10.1016/j.apcata.2015.02.037-
dc.relationinfo:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S0926860X15001350?via%3Dihub-
dc.rightsinfo:eu-repo/semantics/restrictedAccess-
dc.rightshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/-
dc.sourcereponame:CONICET Digital (CONICET)-
dc.sourceinstname:Consejo Nacional de Investigaciones Científicas y Técnicas-
dc.sourceinstacron:CONICET-
dc.subjectRu CATALYSTS-
dc.subjectETS-10-
dc.subjectDRY REFORMING OF METHANE-
dc.subjectHYDROGEN PRODUCTION-
dc.subjectOtras Ingeniería Química-
dc.subjectIngeniería Química-
dc.subjectINGENIERÍAS Y TECNOLOGÍAS-
dc.titleInfluence of La incorporation on the catalytic activity of Ru/ETS-10 catalysts for hydrogen production-
dc.typeinfo:eu-repo/semantics/article-
dc.typeinfo:eu-repo/semantics/publishedVersion-
dc.typeinfo:ar-repo/semantics/articulo-
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