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dc.provenanceCONICET-
dc.creatorAligia, Armando Angel-
dc.date2016-02-01T19:03:20Z-
dc.date2016-02-01T19:03:20Z-
dc.date2013-08-
dc.date2016-03-30 10:35:44.97925-03-
dc.date.accessioned2019-04-29T15:48:06Z-
dc.date.available2019-04-29T15:48:06Z-
dc.date.issued2013-08-
dc.identifierAligia, Armando Angel; Effect of covalency and interactions on the trigonal splitting in Na x CoO2; American Physical Society; Physical Review B; 88; 7; 8-2013; 75-128-
dc.identifier1098-0121-
dc.identifierhttp://hdl.handle.net/11336/3939-
dc.identifier.urihttp://rodna.bn.gov.ar:8080/jspui/handle/bnmm/302388-
dc.descriptionWe calculate the effective trigonal crystal field Delta that splits the t2g levels of effective models for Nax CoO2 as the local symmetry around a Co ion is reduced from Oh to D3d . To this end, we solve numerically a CoO6 cluster containing a Co ion with all 3d states and their interactions included, and its six nearest-neighbor O atoms, with the geometry of the system, in which the CoO6 octahedron is compressed along a C3 axis. We obtain Delta≈ 130 meV, with the sign that agrees with previous quantum chemistry calculations but disagrees with first-principles results in the local density approximation (LDA). We find that Delta is very sensitive to a Coulomb parameter that controls the Hund coupling and charge distribution among the d orbitals. The origin of the discrepancy with LDA results is discussed.-
dc.descriptionFil: Aligia, Armando Angel. Comisión Nacional de Energía Atómica. Gerencia del Area de Investigación y Aplicaciones No Nucleares. Gerencia de Física (Centro Atómico Bariloche); Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Patagonia Norte; Argentina-
dc.formatapplication/pdf-
dc.formatapplication/pdf-
dc.languageeng-
dc.publisherAmerican Physical Society-
dc.relationinfo:eu-repo/semantics/altIdentifier/url/http://journals.aps.org/prb/abstract/10.1103/PhysRevB.88.075128-
dc.relationinfo:eu-repo/semantics/altIdentifier/arxiv/1308.5162-
dc.relationinfo:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.88.075128-
dc.relationinfo:eu-repo/semantics/altIdentifier/url/http://arxiv.org/abs/1308.5162-
dc.relationinfo:eu-repo/semantics/altIdentifier/issn/1098-0121-
dc.relationinfo:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1103/PhysRevB.88.075128-
dc.rightsinfo:eu-repo/semantics/openAccess-
dc.rightshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/-
dc.sourcereponame:CONICET Digital (CONICET)-
dc.sourceinstname:Consejo Nacional de Investigaciones Científicas y Técnicas-
dc.sourceinstacron:CONICET-
dc.source.urihttp://hdl.handle.net/11336/3939-
dc.subjectCovalency-
dc.subjectInteractions-
dc.subjectSplitting-
dc.subjectNaxCoO2-
dc.subjectFísica de los Materiales Condensados-
dc.subjectCiencias Físicas-
dc.subjectCIENCIAS NATURALES Y EXACTAS-
dc.titleEffect of covalency and interactions on the trigonal splitting in Na x CoO2-
dc.typeinfo:eu-repo/semantics/article-
dc.typeinfo:eu-repo/semantics/publishedVersion-
dc.typeinfo:ar-repo/semantics/articulo-
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