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dc.creatorBorosky, Gabriela Leonor-
dc.creatorLaali, Kenneth K.-
dc.date2018-10-10T17:27:06Z-
dc.date2018-10-10T17:27:06Z-
dc.date2012-08-
dc.date2018-09-18T16:16:29Z-
dc.date.accessioned2019-04-29T15:51:06Z-
dc.date.available2019-04-29T15:51:06Z-
dc.date.issued2012-08-
dc.identifierBorosky, Gabriela Leonor; Laali, Kenneth K.; In Silico study of carcinogenic o-Quinone metabolites derived from polycyclic aromatic hydrocarbons (PAHs); John Wiley & Sons Ltd; Journal Of Physical Organic Chemistry; 25; 8; 8-2012; 720-728-
dc.identifier0894-3230-
dc.identifierhttp://hdl.handle.net/11336/62085-
dc.identifierCONICET Digital-
dc.identifierCONICET-
dc.identifier.urihttp://rodna.bn.gov.ar:8080/jspui/handle/bnmm/303703-
dc.descriptionA computational density functional theory study on the structural and electronic properties of several polycyclic aromatic hydrocarbon (PAH) ortho-quinones was performed and the possible mechanism of DNA-adduct formation was analyzed to evaluate its thermodynamic viability. Molecular docking techniques were applied to examine the noncovalent interactions developed when a model PAH ortho-quinone intercalates between the DNA double helix. Quantum-chemical ONIOM (our Own N-layer Integrated molecular Orbital molecular Mechanics) calculations within the structure of a DNA fragment were carried out to evaluate the significant steps of noncovalent complex and covalent adduct formation. The solvent effect was also considered by employing a continuum solvation model. The present calculations suggest that initial noncovalent interactions of the PAH o-quinone within the DNA double helix could determine the feasibility of benzo[a]pyrene-7,8-dione-DNA covalent adduct formation, and that dispersion-corrected functionals are more suitable for locating the noncovalent complex. Copyright © 2012 John Wiley & Sons, Ltd.-
dc.descriptionFil: Borosky, Gabriela Leonor. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina. University of North Florida; Estados Unidos-
dc.descriptionFil: Laali, Kenneth K.. University of North Florida; Estados Unidos-
dc.formatapplication/pdf-
dc.formatapplication/pdf-
dc.languageeng-
dc.publisherJohn Wiley & Sons Ltd-
dc.relationinfo:eu-repo/semantics/altIdentifier/doi/https://dx.doi.org/10.1002/poc.2924-
dc.relationinfo:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/abs/10.1002/poc.2924-
dc.rightsinfo:eu-repo/semantics/restrictedAccess-
dc.rightshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/-
dc.sourcereponame:CONICET Digital (CONICET)-
dc.sourceinstname:Consejo Nacional de Investigaciones Científicas y Técnicas-
dc.sourceinstacron:CONICET-
dc.subjectBIOACTIVATION PATHWAYS-
dc.subjectMOLECULAR DOCKING-
dc.subjectONIOM-
dc.subjectORTHO-QUINONES-
dc.subjectOUR OWN N-LAYER INTEGRATED MOLECULAR ORBITAL MOLECULAR MECHANICS CALCULATIONS-
dc.subjectPOLYCYCLIC AROMATIC HYDROCARBONS-
dc.subjectOtras Ciencias Químicas-
dc.subjectCiencias Químicas-
dc.subjectCIENCIAS NATURALES Y EXACTAS-
dc.titleIn Silico study of carcinogenic o-Quinone metabolites derived from polycyclic aromatic hydrocarbons (PAHs)-
dc.typeinfo:eu-repo/semantics/article-
dc.typeinfo:eu-repo/semantics/publishedVersion-
dc.typeinfo:ar-repo/semantics/articulo-
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